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  • 标题:Effect of the fluid shear rate on the induction time of CO2‐THF hydrate formation
  • 本地全文:下载
  • 作者:Sélim Douïeb ; Sélim Douïeb ; Simon Archambault
  • 期刊名称:Canadian Journal of Chemical Engineering
  • 印刷版ISSN:0008-4034
  • 出版年度:2017
  • 卷号:95
  • 期号:1
  • 页码:187-198
  • DOI:10.1002/cjce.22650
  • 语种:English
  • 出版社:Chemical Institute of Canada
  • 摘要:Abstract A method that allows the effect of the fluid shear rate on the induction time of gas hydrate formation to be characterized was developed and applied to CO2‐THF hydrate formation. The investigation of the effect of the application of a constant shear rate (50 to 300 s−1) to the liquid phase from which the hydrates are formed revealed that the mean induction time decreases significantly as the applied shear rate increases. This could primarily be attributed to a decrease in the time required for stable gas hydrate nuclei to be generated and to grow to a macroscopically detectable size. The induction time could also be significantly reduced by the application of a high shear rate (900 s−1) to the liquid phase for a relatively short, defined period of time.
  • 关键词:encrystallizationgas hydratesinduction timeshear rateCouette‐Taylor
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