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  • 标题:Spin glass behavior and magnetic boson peak in a structural glass of a magnetic ionic liquid
  • 本地全文:下载
  • 作者:Maiko Kofu ; Ryuta Watanuki ; Toshiro Sakakibara
  • 期刊名称:Scientific Reports
  • 电子版ISSN:2045-2322
  • 出版年度:2021
  • 卷号:11
  • DOI:10.1038/s41598-021-91619-z
  • 语种:English
  • 出版社:Springer Nature
  • 摘要:Glassy magnetic behavior has been observed in a wide range of crystalline magnetic materials called spin glass. Here, we report spin glass behavior in a structural glass of a magnetic ionic liquid, C4mimFeCl 4. Magnetization measurements demonstrate that an antiferromagnetic ordering occurs at T N  = 2.3 K in the crystalline state, while a spin glass transition occurs at T SG  = 0.4 K in the structural glass state. In addition, localized magnetic excitations were found in the spin glass state by inelastic neutron scattering, in contrast to spin-wave excitations in the ordered phase of the crystalline sample. The localized excitation was scaled by the Bose population factor below T SG and gradually disappeared above T SG. This feature is highly reminiscent of boson peaks commonly observed in structural glasses. We suggest the “magnetic” boson peak to be one of the inherent dynamics of a spin glass state.
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