标题：Using a New Top‐Down Constrained Emissions Inventory to Attribute the Previously Unknown Source of Extreme Aerosol Loadings Observed Annually in the Monsoon Asia Free Troposphere
摘要：The contribution of biomass burning to the total aerosol loading over Monsoon Asia is both significant and continuing to increase. To better match the spatio‐temporal distribution of aerosols and trace gasses observed in the free troposphere, this work applied a 3‐D constrained emission inventory based on top‐down remotely sensed NO2 measurement to investigate the most extreme of the annually occurring biomass burning seasons in Monsoon Asia. In 2016, this constituted an extreme event observed over a 6‐day period covering millions of square kilometers, including over regions that are typically in the rainy phase of the Asian Monsoon. The results are shown to be consistent with respect to Tropical Rainfall Measuring Mission precipitation, AERONET measurements, MODIS AOD, MOPITT CO, and reanalysis meteorology, over both the biomass burning source as well as the millions of square kilometers downwind both to the East and to the Southwest. Reproducing the observed long‐range transport pattern requires the time of biomass burning to be increased, regions not previously identified as burning to be actual source regions, and the emissions of Black Carbon (BC) to be 6.6 to 11.9 times larger than current inventories. The underlying mechanism for this long‐range transport involves a new 3‐D pathway that can occur during the transition from the North phase to the South phase of the Asian Monsoon. The results are also consistent with the new idea that large loadings of BC in the lower free troposphere may significantly affect the meteorological field and the overall vertical distribution of aerosols in the tropical troposphere.
