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  • 标题:Preparation of hexagonal nanoporous Al 2O 3/TiO 2/TiN as a novel photodetector with high efficiency
  • 本地全文:下载
  • 作者:Asmaa M. Elsayed ; Mohamed Rabia ; Mohamed Shaban
  • 期刊名称:Scientific Reports
  • 电子版ISSN:2045-2322
  • 出版年度:2021
  • 卷号:11
  • DOI:10.1038/s41598-021-96200-2
  • 语种:English
  • 出版社:Springer Nature
  • 摘要:The unique optical properties of metal nitrides enhance many photoelectrical applications. In this work, a novel photodetector based on TiO 2/TiN nanotubes was deposited on a porous aluminum oxide template (PAOT) for light power intensity and wavelength detection. The PAOT was fabricated by the Ni-imprinting technique through a two-step anodization method. The TiO 2/TiN layers were deposited by using atomic layer deposition and magnetron sputtering, respectively. The PAOT and PAOT/TiO 2/TiN were characterized by several techniques such as X-ray diffraction (XRD), scanning electron microscope (SEM), and energy dispersive X-ray (EDX). The PAOT has high-ordered hexagonal nanopores with dimensions ~ 320 nm pore diameter and ~ 61 nm interpore distance. The bandgap of PAOT/TiO 2 decreased from 3.1 to 2.2 eV with enhancing absorption of visible light after deposition of TiN on the PAOT/TiO 2. The PAOT/TiO 2/TiN as photodetector has a responsivity (R) and detectivity (D) of 450 mAW -1 and 8.0 × 10 12 Jones, respectively. Moreover, the external quantum efficiency (EQE) was 9.64% at 62.5 mW.cm −2 and 400 nm. Hence, the fabricated photodetector (PD) has a very high photoelectrical response due to hot electrons from the TiN layer, which makes it very hopeful as a broadband photodetector.
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