摘要：SummaryDespite great progress in battery safety modeling, accurately predicting the evolution of multiphysics systems is extremely challenging. The question on how to ensure safety of billions of automotive batteries during their lifetime remains unanswered. In this study, we overcome the challenge by developing machine learning techniques based on the recorded data that are uploaded to the cloud. Using charging voltage and temperature curves from early cycles that are yet to exhibit symptoms of battery failure, we apply data-driven models to both predict and classify the sample data by health condition based on the observational, empirical, physical, and statistical understanding of the multiscale systems. The best well-integrated machine learning models achieve a verified classification accuracy of 96.3% (exhibiting an increase of 20.4% from initial model) and an average misclassification test error of 7.7%. Our findings highlight the need for cloud-based artificial intelligence technology tailored to robustly and accurately predict battery failure in real-world applications.Graphical abstractDisplay OmittedHighlights•A well-integrated machine learning technique is applied to failure prediction•A cloud-based closed-loop framework is established for real-world EV applications•Cloud-based AI solution is based on an in-depth analysis of the field data•Both electrochemical and statistical feature engineering are establishedElectrochemistry; Electrochemical energy storage; Computational materials science
