Photo- and electron-sensitivities of K2 [Cu (C2O4) 2]·2H2O and CuC2O4·1/2H2O were studied by measuring the variation of reflection density upon radiation with ultraviolet light and electron beam. K2 [Cu (C2O4) 2]·2H2O is thermally developable. Its photographic sensitivities which were measured as radiation energy required to obtain D =0.1 above fog, are 2.2×106erg/cm2 at 254 nm and 1.6×107erg/cm2 at 334 nm after development. Electron sensitivities measured in the same way are 3.5×10-7 and 2.4×10-6 C/cm2 for K2 [Cu (C2O4) 2]·2H2O after development and CuC2O4·1/2H2O, respectively. The influence of several binders on the photographic sensitivity of CuC2O4·1/2H2O was studied for both ultraviolet light and electron beam radiations. The sensitivity was found to be inversely proportional to the permeability of oxygen into binder film. Cu2O was found to be one of the photolysis products of either of the two compounds.