首页    期刊浏览 2024年11月08日 星期五
登录注册

文章基本信息

  • 标题:理論計算によるテトラアリールエテン類の構造解析と光異性化
  • 本地全文:下载
  • 作者:山本 岳郎 ; 大田 義広 ; 鈴木 麻衣実
  • 期刊名称:日本写真学会誌
  • 印刷版ISSN:0369-5662
  • 电子版ISSN:1884-5932
  • 出版年度:2004
  • 卷号:67
  • 期号:Suppliment1
  • 页码:126-127
  • DOI:10.11454/photogrst1964.67.Suppliment1_126
  • 出版社:The Society of Photographic Science and Technolgy of Japan
  • 摘要:

    Photo-induced isomerization of 1, 2-di (3-aminophenyl)-1, 2-diphenylethene contains following reactions; 1) rotation of m -aminophenyl groups, 2) epimerization, 3) rotation of C=C double bond part. The details of these reaction processes were investigated by means of DFT calculation (B3LYP) with LANL2DZ basis set. The activation energies for the rotation of C-C single bond of m -aminophenyl group and for the epimarization of the molecule were 8.8 kcal/mol and 7.9 kcal/mol, respectively. Although large activation energy requires for the rotation of the C=C double bond at singlet states, C=C double bond lengthen and close to rotatable C-C single bond with radical on each carbons at trilet states.

国家哲学社会科学文献中心版权所有