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  • 标题:Unusual ferromagnetic critical behavior owing to short-range antiferromagnetic correlations in antiperovskite Cu1-xNMn3+x (0.1 ≤ x ≤ 0.4)
  • 本地全文:下载
  • 作者:Jianchao Lin ; Peng Tong ; Dapeng Cui
  • 期刊名称:Scientific Reports
  • 电子版ISSN:2045-2322
  • 出版年度:2015
  • 卷号:5
  • DOI:10.1038/srep07933
  • 出版社:Springer Nature
  • 摘要:For ferromagnets, varying from simple metals to strongly correlated oxides,the critical behaviors near the Curie temperature ( T C) can be grouped into several universal classes. In this paper, we report an unusual critical behavior in manganese nitrides Cu1- x NMn3+ x (0.1 ≤ x ≤ 0.4). Although the critical behavior below T C can be well described by mean field (MF) theory, robust critical fluctuations beyond the expectations of any universal classes are observed above T C in x = 0.1. The critical fluctuations become weaker when x increases, and the MF-like critical behavior is finally restored at x = 0.4. In addition, the paramagnetic susceptibility of all the samples deviates from the Curie-Weiss (CW) law just above T C. This deviation is gradually smeared as x increases. The short-range antiferromagnetic ordering above T C revealed by our electron spin resonance measurement explains both the unusual critical behavior and the breakdown of the CW law.
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