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  • 标题:Hydrogen Production from Water by Photolysis, Sonolysis and Sonophotolysis with Solid Solutions of Rare Earth, Gallium and Indium Oxides as Heterogeneous Catalysts
  • 本地全文:下载
  • 作者:Penconi, Marta ; Rossi, Federico ; Ortica, Fausto
  • 期刊名称:Sustainability
  • 印刷版ISSN:2071-1050
  • 出版年度:2015
  • 卷号:7
  • 期号:7
  • 页码:9310-9325
  • 出版社:MDPI, Open Access Journal
  • 摘要:In this work, we present the hydrogen production by photolysis, sonolysis and sonophotolysis of water in the presence of newly synthesized solid solutions of rare earth, gallium and indium oxides playing as catalysts. From the experiments of photolysis, we found that the best photocatalyst is the solid solution Y 0.8 Ga 0.2 InO 3 doped by sulphur atoms. In experiments of sonolysis, we optimized the rate of hydrogen production by changing the amount of water, adding ethanol and tuning the power of our piezoelectric transducer. Finally, we performed sonolysis and sonophotolysis experiments in the presence of S:Y 0.8 Ga 0.2 InO 3 finding a promising synergistic effect of UV-visible electromagnetic waves and 38 kHz ultrasound waves in producing H 2 .
  • 关键词:hydrogen energy; solar energy; photocatalysis; sonochemistry; synergy; metal oxides; sulphur-doping
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