期刊名称：Proceedings of the National Academy of Sciences
印刷版ISSN：0027-8424
电子版ISSN：1091-6490
出版年度：2010
卷号：107
期号：24
页码：10810-10814
DOI：10.1073/pnas.0913605107
语种：English
出版社：The National Academy of Sciences of the United States of America
摘要：Recent high precision 142Nd isotope measurements showed that global silicate differentiation may have occurred as early as 30-75 Myr after the Solar System formation [Bennett V, et al. (2007) Science 318:1907-1910]. This time scale is almost contemporaneous with Earth's core formation at [~]30 Myr [Yin Q, et al. (2002) Nature 418:949-952]. The 182Hf-182W system provides a powerful complement to the 142Nd results for early silicate differentiation, because both core formation and silicate differentiation fractionate Hf from W. Here we show that eleven terrestrial samples from diverse tectonic settings, including five early Archean samples from Isua, Greenland, of which three have been previously shown with 142Nd anomalies, all have a homogeneous W isotopic composition, which is [~]2{varepsilon}-unit more radiogenic than the chondritic value. By using a 3-stage model calculation that describes the isotopic evolution in chondritic reservoir and core segregation, as well as silicate differentiation, we show that the W isotopic composition of terrestrial samples provides the most stringent time constraint for early core formation (27.5-38 Myr) followed by early terrestrial silicate differentiation (38-75 Myr) that is consistent with the terrestrial 142Nd anomalies.
关键词：hafnium ; tungsten ; hidden reservoir ; Hawaii ; Iceland
