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  • 标题:High efficiency and low roll-off green OLEDs with simple structure by utilizing thermally activated delayed fluorescence material as the universal host
  • 本地全文:下载
  • 作者:Bo Zhao ; Yanqin Miao ; Zhongqiang Wang
  • 期刊名称:Nanophotonics
  • 印刷版ISSN:2192-8606
  • 电子版ISSN:2192-8614
  • 出版年度:2017
  • 卷号:6
  • 期号:5
  • 页码:1133-1140
  • DOI:10.1515/nanoph-2016-0177
  • 出版社:Walter de Gruyter GmbH
  • 摘要:

    We achieved high-efficiency and low-roll-off green fluorescent and phosphorescent organic light-emitting diodes (OLEDs) simultaneously by adopting the thermally activated delayed fluorescence material of bis[4-(9,9-dimethyl-9,10-dihydroacridine)phenyl]sulfone as the universal host. At a luminance of 1000 cd/m2, fluorescent OLEDs based on C545T get a current efficiency, power efficiency, and external quantum efficiency (EQE) of 31.8 cd/A, 25.0 lm/W, and 9.26%, respectively. This is almost the highest efficiency based on C545T at the luminance of 1000 cd/m2 to date. On the other hand, phosphorescent OLEDs with Ir(ppy)3 as the emitter realize a maximum current efficiency, power efficiency, and EQE of 64.3 cd/A, 62.4 lm/W, and 18.5%, respectively. More important, the EQE remains 17.8% at the representative luminance of 1000 cd/m2 and the roll-off ratio is just 3.78%. The transient photoluminescence decay measurement demonstrates that the up-conversion of host triplet excitons plays a key role in the high efficiency and low roll-off. More detailed discussions are also given.

  • 关键词:OLEDs ; DMAC-DPS ; TADF ; roll-off
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