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  • 标题:Mixed-order phase transition in a colloidal crystal
  • 本地全文:下载
  • 作者:Ricard Alert ; Pietro Tierno ; Jaume Casademunt
  • 期刊名称:Proceedings of the National Academy of Sciences
  • 印刷版ISSN:0027-8424
  • 电子版ISSN:1091-6490
  • 出版年度:2017
  • 卷号:114
  • 期号:49
  • 页码:12906-12909
  • DOI:10.1073/pnas.1712584114
  • 语种:English
  • 出版社:The National Academy of Sciences of the United States of America
  • 摘要:Mixed-order phase transitions display a discontinuity in the order parameter like first-order transitions yet feature critical behavior like second-order transitions. Such transitions have been predicted for a broad range of equilibrium and nonequilibrium systems, but their experimental observation has remained elusive. Here, we analytically predict and experimentally realize a mixed-order equilibrium phase transition. Specifically, a discontinuous solid–solid transition in a 2D crystal of paramagnetic colloidal particles is induced by a magnetic field H . At the transition field H s , the energy landscape of the system becomes completely flat, which causes diverging fluctuations and correlation length ξ ∝ | H 2 − H s 2 | − 1 / 2 . Mean-field critical exponents are predicted, since the upper critical dimension of the transition is d u = 2 . Our colloidal system provides an experimental test bed to probe the unconventional properties of mixed-order phase transitions.
  • 关键词:phase transitions ; critical phenomena ; colloidal crystals
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