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  • 标题:One-step synthesis of nitrogen and chlorine co-doped fluorescent carbon nanodots for the sensitive detection of Ag+
  • 作者:C Huang ; H Y Liu ; M Z Zhang
  • 期刊名称:IOP Conference Series: Earth and Environmental Science
  • 印刷版ISSN:1755-1307
  • 电子版ISSN:1755-1315
  • 出版年度:2018
  • 卷号:186
  • 期号:2
  • 页码:012027
  • DOI:10.1088/1755-1315/186/2/012027
  • 语种:English
  • 出版社:IOP Publishing
  • 摘要:Nitrogen and chlorine co-doped fluorescent carbon nanodots (CDs) were prepared using a facile and eco-friendly solvothermal process in which N-Chlorosuccinimide(NCS) was used as a carbon source. The resulting CDs were characterized by UV-visible absorption spectroscopy, fluorescence spectroscopy, high-resolution transmission electron microscopy (HR-TEM), Fourier transform infrared and X-ray photoelectron spectroscopy (XPS). It shows emission of blue light at 410 nm when excited at 340 nm. High quantum yield of 21.7% and good biocompatibility were also observed. Importantly, the fluorescence intensity of CDs was selectively quenched after addition of Ag+. Based upon the aforementioned phenomenon, a new fluorescent biosensor for the detection of Ag+ was proposed. The linear range and detection limit was 5-70 μM and 1.06 μM, respectively. Eventually, these superior properties demonstrated that the CDs have promising applications in the field of environmental and biomedicine research.
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