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  • 标题:Reconstructing charge-carrier dynamics in porous silicon membranes from time-resolved interferometric measurements
  • 本地全文:下载
  • 作者:Wei He ; Rihan Wu ; Igor V. Yurkevich
  • 期刊名称:Scientific Reports
  • 电子版ISSN:2045-2322
  • 出版年度:2018
  • 卷号:8
  • 期号:1
  • 页码:17172
  • DOI:10.1038/s41598-018-35210-z
  • 语种:English
  • 出版社:Springer Nature
  • 摘要:We performed interferometric time-resolved simultaneous reflectance and transmittance measurements to investigate the carrier dynamics in pump-probe experiments on thin porous silicon membranes. The experimental data was analysed by using a method built on the Wentzel-Kramers-Brillouin approximation and the Drude model, allowing us to reconstruct the excited carriers' non-uniform distribution in space and its evolution in time. The analysis revealed that the carrier dynamics in porous silicon, with ~50% porosity and native oxide chemistry, is governed by the Shockley-Read-Hall recombination process with a characteristic time constant of 375 picoseconds, whereas diffusion makes an insignificant contribution as it is suppressed by the high rate of scattering.
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