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  • 标题:Versatile chemical handling to confine radioactive cesium as stable inorganic crystal
  • 本地全文:下载
  • 作者:Nguyen Duy Quang ; Hiromi Eba ; Kenji Sakurai
  • 期刊名称:Scientific Reports
  • 电子版ISSN:2045-2322
  • 出版年度:2018
  • 卷号:8
  • 期号:1
  • 页码:15051
  • DOI:10.1038/s41598-018-32943-9
  • 语种:English
  • 出版社:Springer Nature
  • 摘要:), which is promising as a form of the final storage. In this processing, the clays are used as a source for aluminum and silicon, and it is important to get a well-mixed homogenous solution by the aid of some heat and pressure. The present method proposes the use of ethylene glycol as a solvent, rather than water. It has been found that one can obtain crystalline pollucite by heating up to 350 °C in a high-pressure container (~15 MPa), mixed with montmorillonite - an abundant natural clay and ethylene glycol. It has been found that the reduction of the amount of water helps to achieve very high confinement rate in a reasonable time of few~20 h. This will be fairly important in processing contaminated water in the nuclear power plant. The influence of seawater has been also examined.
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