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  • 标题:Electron pair escape from fullerene cage via collective modes
  • 本地全文:下载
  • 作者:Michael Schüler ; Yaroslav Pavlyukh ; Paola Bolognesi
  • 期刊名称:Scientific Reports
  • 电子版ISSN:2045-2322
  • 出版年度:2016
  • 卷号:6
  • 期号:1
  • DOI:10.1038/srep24396
  • 语种:English
  • 出版社:Springer Nature
  • 摘要:Experiment and theory evidence a new pathway for correlated two-electron release from many-body compounds following collective excitation by a single photon. Using nonequilibrium Green's function approach we trace plasmon oscillations as the key ingredient of the effective electron-electron interaction that governs the correlated pair emission in a dynamic many-body environment. Results from a full ab initio implementation for C60 fullerene are in line with experimental observations. The findings endorse the correlated two-electron photoemission as a powerful tool to access electronic correlation in complex systems.
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