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  • 标题:Improving Photocatalytic Performance from Bi2WO6@MoS2/graphene Hybrids via Gradual Charge Transferred Pathway
  • 本地全文:下载
  • 作者:Ming Liu ; Xin Xue ; Shansheng Yu
  • 期刊名称:Scientific Reports
  • 电子版ISSN:2045-2322
  • 出版年度:2017
  • 卷号:7
  • 期号:1
  • DOI:10.1038/s41598-017-03911-6
  • 语种:English
  • 出版社:Springer Nature
  • 摘要:The charge transfer from the main catalyst to the cocatalyst is a key factor to enhance catalytic activity for photocatalytic nanocomposite materials. In order to enhance the charge transfer between Bi2WO6 and graphene, we inlet MoS2 as a "stepping-stone" into Bi2WO6 and graphene. Here, we report an effective strategy to synthesize ternary Bi2WO6@MoS2/graphene nanocomposite photocatalyst by a facile two-step hydrothermal method, which is afforded by assembling two cocatalysts, graphene and MoS2, into the Bi2WO6 matrix with a nanoparticle morphology as a visible light harvester. Compared with Bi2WO6/graphene, Bi2WO6/MoS2 and pure Bi2WO6, the Bi2WO6@MoS2/graphene ternary composites exhibit superior photocatalytic activity owing to an enhanced charge carrier separation via gradual charge transferred pathway. This work indicates a promising cocatalyst strategy for designing a more efficient graphene based semiconductor photocatalyst toward degradation of organic pollutants.
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