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  • 标题:Non-noble metal based broadband photothermal absorbers for cost effective interfacial solar thermal conversion
  • 本地全文:下载
  • 作者:Han Gong ; Xin Liu ; Guoliang Liu
  • 期刊名称:Nanophotonics
  • 印刷版ISSN:2192-8606
  • 电子版ISSN:2192-8614
  • 出版年度:2020
  • 卷号:9
  • 期号:6
  • 页码:1539-1546
  • DOI:10.1515/nanoph-2020-0168
  • 出版社:Walter de Gruyter GmbH
  • 摘要:In recent years, noble metal-based solar absorbers have been extensively studied as their pronounced plasmonic resonances and high solar-to-thermal conversion efficiency. However, the high cost of noble metals is the unavoidable roadblock restricting the way towards scalability. In this work, we report a nickel-based photothermal absorbers, which is capable of realizing an average solar absorption of ∼97% in the range of 400–2500 nm originating from relatively weaker collective plasmonic resonances but more pronounced single electron excitation. Importantly, it is easily fabricated via the straightforward physical deposition and cost-effective with a raw material price of ∼0.3% gold and ∼20% of silver. We used it for interfacial solar vapor generation and realized an evaporation rate of ∼0.9 kg m −2  h −1 under one sun, almost comparable to the counterparts made from noble metals. The excellent performance combined with the cost effective and scalable fabrication process makes it be a promising candidate for mass off-grid solar desalination.
  • 关键词:interband transition ; lasmonic absorber ; photothermal conversion ; solar evaporation
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