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  • 标题:MXene-Ti3C2 assisted one-step synthesis of carbon-supported TiO2/Bi4NbO8Cl heterostructures for enhanced photocatalytic water decontamination
  • 本地全文:下载
  • 作者:Daixun Jiang ; Xun Sun ; Xilu Wu
  • 期刊名称:Nanophotonics
  • 印刷版ISSN:2192-8606
  • 电子版ISSN:2192-8614
  • 出版年度:2020
  • 卷号:9
  • 期号:7
  • 页码:2077-2088
  • DOI:10.1515/nanoph-2020-0088
  • 出版社:Walter de Gruyter GmbH
  • 摘要:The strategy to improve the photocatalytic removal efficiencies towards organic pollutants is still a challenge for the novel Sillen–Aurivillius perovskite type Bi4 NbO8 Cl. Herein, we report carbon-supported TiO2 /Bi4 NbO8 Cl (C-TiO2 /Bi4 NbO8 Cl) heterostructures with enhanced charge separation efficiency, which were fabricated via molten-salt flux process. The carbon-supported TiO2 particles were derived from MXene Ti3 C2 precursors, and attached on plate-like Bi4 NbO8 Cl, acting as electron-traps to achieve supressed recombination of photo-induced charges. The improved charge separation confers C-TiO2 /Bi4 NbO8 Cl heterostructures superior photocatalytic performance with 53% higher than pristine Bi4 NbO8 Cl, towards rhodamine B removal with the help of photo-induced holes. Moreover, the C-TiO2 /Bi4 NbO8 Cl heterostructures can be expanded to deal with other water contaminants, such as methyl orange, ciprofloxacin and 2,4-dichlorophenol with 44, 25 and 13% promotion, respectively, and thus the study offers a series of efficient photocatalysts for water purification.
  • 关键词:Bi4NbO8Cl ; heterostructures ; MXene Ti3C2 ; photocatalysis
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