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  • 标题:Aerosol Particles from Dried Salt-Lakes and Saline Soils Carried on Dust Storms over Beijing
  • 本地全文:下载
  • 作者:Xingying Zhang ; Guoshun Zhuang ; Hui Yuan
  • 期刊名称:Terrestrial Atmospheric and Oceanic Sciences
  • 印刷版ISSN:1017-0839
  • 出版年度:2009
  • 卷号:20
  • 期号:4
  • 页码:619-628
  • DOI:10.3319/TAO.2008.07.11.03(A)
  • 出版社:Chinese Geoscience Union
  • 摘要:Characteristics of individual particles from a super dust storm (DS) on 20 March 2002, and those of non dust storm aero sols for Beijing (NDS) and Duolun (DL) (a desert area) are determined using a variety of methods. In China, typically the source of aero sols in dust storms is thought to be deserts with alumino silicates being the main constituent particles; how ever, this does not reflect a complete analysis with our evidence indicating potential alternate dust sources along the storm¡¦s trans port path. Individual particle anal y sis of aero sols collected from a super dust storm on 20 March 2002 in Beijing shows that among all the 14 elements measured, only S and Cl have re mark able positive correlation. 82.5% of all particles measured contained both S and Cl, and the relative mass per cent age of S and Cl in these particles is much higher than the average of all particles. 62.0% of all particles contained S, Cl, and Na, in which the concentration of Na is 1.4 times higher than average. PMF (Positive Matrix Factorization) anal y sis indicates that NaCl and Na2SO4 are major components of these particles with S and Cl showing significant positive correlation. More over, SO4 2- and Cl- also show significant positive correlation in bulk aero sol analysis. XPS (X-ray Pho to electron Spectros copy) analysis of the surface of aero sols demonstrates that concentrations of Na and S on particles from the dust storm are higher than those from non-dust storm particles in Beijing and also for particles from. It is very likely that particles enriched with S, Cl, and Na is from the surface soils of dried salt-lakes and saline soils enriched with chloride and sulfate. This evidence demonstrates that be sides deserts, surface soils from dry salt-lakes and saline soils of arid and semi-arid areas are also sources of particulates in dust storms over Beijing.
  • 关键词:Dust storm; Individual particle analysis; Correlation of S/Cl; Salt lake and saline soil;
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