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  • 标题:Charge Recombination Kinetics of Bacterial Photosynthetic Reaction Centres Reconstituted in Liposomes: Deterministic Versus Stochastic Approach
  • 本地全文:下载
  • 作者:Emiliano Altamura ; Paola Albanese ; Pasquale Stano
  • 期刊名称:Data
  • 印刷版ISSN:2306-5729
  • 出版年度:2020
  • 卷号:5
  • 期号:2
  • 页码:53-67
  • DOI:10.3390/data5020053
  • 出版社:MDPI Publishing
  • 摘要:In this theoretical work, we analyse the kinetics of charge recombination reaction after a light excitation of the Reaction Centres extracted from the photosynthetic bacterium Rhodobacter sphaeroides and reconstituted in small unilamellar phospholipid vesicles.Due to the compartmentalized nature of liposomes, vesicles may exhibit a random distribution of both ubiquinone molecules and the Reaction Centre protein complexes that can produce significant differences on the local concentrations from the average expected values.Moreover, since the amount of reacting species is very low in compartmentalized lipid systems the stochastic approach is more suitable to unveil deviations of the average time behaviour of vesicles from the deterministic time evolution.
  • 关键词:reaction centres; liposomes; charge recombination; ODE; stochastic simulations
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