摘要：Solar radiation management with stratospheric sulfur aerosols has been proposed as a potential geoengineering strategy to reduce global warming. However, there has been very little investigation on the efficiency of specific injection methods suggested. Here, we show that using stratospheric passenger flights to inject sulfate aerosols would not cause significant forcing under realistic injection scenarios: even if all present-day intercontinental flights were lifted above the tropopause, we simulate global surface shortwave radiative forcings of − 0.05 W m−2 and − 0.10 W m−2 with current and five times enhanced fuel sulfur concentrations, respectively. In the highly unlikely scenario that fuel sulfur content is enhanced by a factor of 50 (i.e. ten times the current legal limit) the radiative forcing is − 0.85 W m−2. This is significantly lower than if the same amount of sulfur were injected over the tropics ( − 1.32 W m−2, for 3 Tg (S) yr−1) due to a faster loss rate and lower intensity of solar radiation in the northern midlatitudes where current flight paths are concentrated. We also predict lower global forcing in northern hemisphere winter than in summer due to the seasonalities of the solar radiation intensity at midlatitudes, the related OH chemistry that produces sulfate aerosol, and removal of particles.
