A computer program has been developed for neutron energy spectrum adjustment using the deconvolution method. The BUNKI-based algorithm has been implemented to converge quickly yielding calculated neutron energy spectrum which is in good agreement with theoretical predictions. The foil activation data have been used as an input for each unfolding technique and various activation foils including Au-197, Al-27, Ni-58, Co-59, and Mg-24 covering thermal to fast energy range have been utilized. The group cross-section values were derived from the data given in the pre-processed cross-section libraries in ENDF-6 format of IRDF-90/NMF-G. Firstly, virtual approach was used for neutron energy spectrum adjustment. In this case, the activity of foils before and after the adjustment was almost the same but the flux had the maximum error of 14%. Secondly, the experimental measured activity of the threshold foils was then used for a real system. The activity of the threshold foils before and after the neutron energy adjustment had the maximum error of 33%.